Comparing results of X-ray diffraction, µ-Raman spectroscopy and neutron diffraction when identifying chemical phases in seized nuclear material, during a comparative nuclear forensics exercise

نویسندگان

  • Stina Holmgren Rondahl
  • Fabien Pointurier
  • Linnea Ahlinder
  • Henrik Ramebäck
  • Olivier Marie
  • Brice Ravat
  • François Delaunay
  • Emma Young
  • Ned Blagojevic
  • James R. Hester
  • Gordon Thorogood
  • Aubrey N. Nelwamondo
  • Tshepo P. Ntsoane
  • Sarah K. Roberts
  • Kiel S. Holliday
چکیده

This work presents the results for identification of chemical phases obtained by several laboratories as a part of an international nuclear forensic round-robin exercise. In this work powder X-ray diffraction (p-XRD) is regarded as the reference technique. Neutron diffraction produced a superior high-angle diffraction pattern relative to p-XRD. Requiring only small amounts of sample, µ-Raman spectroscopy was used for the first time in this context as a potentially complementary technique to p-XRD. The chemical phases were identified as pure UO2 in two materials, and as a mixture of UO2, U3O8 and an intermediate species U3O7 in the third material.

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عنوان ژورنال:

دوره 315  شماره 

صفحات  -

تاریخ انتشار 2018